Characterization of the Physical and Biodegradation Properties of Biodegradable Plastic from Carboxymethyl Cellulose, Young Coconut Shells and Cassava Starch

Authors

  • Putri Faradilla Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Rini Selly Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Adelia Febriyossa Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Moondra Zubir Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Siti Rahmah Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Dwi Sapri Ramadhan Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia
  • Tesalonika Bela Department of Chemistry, Faculty of Mathematics and Natural Science, Universitas Negeri Medan, North Sumatera, 20221, Indonesia

DOI:

https://doi.org/10.24114/ijcst.v9i1.72442

Keywords:

bioplastic, carboxymethyl cellulose, cassava starch, mechanical properties, biodegradation

Abstract

Biodegradable plastics derived from renewable biomass were synthesized using carboxymethyl cellulose (CMC) isolated from young coconut husk and cassava starch at different CMC:starch ratios (1:1, 1:2, and 2:1). Physical characterization included tensile strength, elongation, Young’s modulus, and water resistance, while biodegradation performance was assessed through a 15-day soil burial test. The tensile strength reached its highest value at a ratio of 2:1 (2.0068 MPa), fulfilling the JIS 2-1707 requirement for biodegradable films. Elongation values were inversely related to CMC content, with the highest elongation (62.69%) observed at the 1:2 ratio. Water resistance was also optimal at the 1:2 ratio, indicating lower hydrophilicity compared to CMC-rich films. Biodegradation tests showed that bioplastics with higher CMC content (2:1) degraded fastest, achieving 97.37% mass loss on day 15. These findings demonstrate that the CMC:starch ratio significantly affects mechanical stability, moisture sensitivity, and biodegradation rate. Overall, the bioplastic films developed in this study exhibit promising properties for eco-friendly and lightweight packaging applications.

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Published

2026-01-31